FIXED-BED ADSORPTION OF AQUEOUS VANILLIN ONTO RESIN H103

Rozaimi Abu Samah

Abstract


The main objective of this work was to design and model fixed bed adsorption column for the adsorption of vanillin from aqueous solution. Three parameters were evaluated for identifying the performance of vanillin adsorption in fixed-bed mode, which were bed height, vanillin initial concentration, and feed flow rate. The maximum adsorption capacity was increased more than threefold to 314.96 mg vanillin/g resin when the bed height was increased from 5 cm to 15 cm. Bohart-Adams model and Belter equation were used for designing fixed-bed column and predicting the performance of the adsorption process. A high value of determination coefficient (R2) of 0.9672 was obtained for the modelling of vanillin adsorption onto resin H103.

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References


G. Reineccius, Flavoring Materials, Flavor Chemistry and Technology, Second Edition, CRC Press, Florida, pp. 203-259, 2005.

J. E. Dolfini, J. Glinka, and A. C. Bosch. Patent No. 4,927,805. Washington: USPTO, 1990.

J.-P. Vidal, Vanillin, Kirk-Othmer Food and Feed Technology, John Wiley & Sons, New Jersey, pp. 526-538, 2008.

N. J. Walton, A. Narbad, C. Faulds, and G. Williamson. "Novel approaches to the biosynthesis of vanillin," Current Opinion in Biotechnology, 11(5), 490-496, 2000.

C. Brazinha, D. S. Barbosa, and J. G. Crespo. "Sustainable recovery of pure natural vanillin from fermentation media in a single pervaporation step," Green Chemistry, 13(8), 2197-2203, 2011.

Y.-T. Wu, M. Feng, W.-W. Ding, X.-Y. Tang, Y.-H. Zhong, and Z.-Y. Xiao. "Preparation of vanillin by bioconversion in a silicon rubber membrane bioreactor," Biochemical Engineering Journal, 41(2), 193-197, 2008.

L. Sciubba, D. Di Gioia, F. Fava, and C. Gostoli. "Membrane-based solvent extraction of vanillin in hollow fiber contactors," Desalination, 241(1), 357-364, 2009.

G. de Brito Cardoso, T. Mourão, F. M. Pereira, M. G. Freire, A. T. Fricks, C. M. F. Soares, and Á. S. Lima. "Aqueous two-phase systems based on acetonitrile and carbohydrates and their application to the extraction of vanillin," Separation and Purification Technology, 104(0), 106-113, 2013.

D. F. Taber, S. Patel, T. M. Hambleton, and E. E. Winkel. "Vanillin synthesis from 4-hydroxybenzaldehyde," Journal of Chemical Education, 84(7), 1158, 2007.

R. Li, Z. Jiang, L. Mao, and H. Shen. "Adsorbed resin phase spectrophotometric determination of vanillin or/and its derivatives," Talanta, 47(5), 1121-1127, 1998.

L.-Q. Zhao, Z.-H. Sun, P. Zheng, and J.-Y. He. "Biotransformation of isoeugenol to vanillin by Bacillus fusiformis CGMCC1347 with the addition of resin HD-8," Process Biochemistry, 41(7), 1673-1676, 2006.

M. Zabkova, M. Otero, M. Minceva, M. Zabka, and A. E. Rodrigues. "Separation of synthetic vanillin at different pH onto polymeric adsorbent Sephabeads SP206," Chemical Engineering and Processing: Process Intensification, 45(7), 598-607, 2006.

D. Hua, C. Ma, L. Song, S. Lin, Z. Zhang, Z. Deng, and P. Xu. "Enhanced vanillin production from ferulic acid using adsorbent resin," Applied Microbiology and Biotechnology, 74(4), 783-790, 2007.

Z. Wang, K. Chen, J. Li, Q. Wang, and J. Guo. "Separation of vanillin and syringaldehyde from oxygen delignification spent liquor by macroporous resin adsorption," CLEAN – Soil, Air, Water, 38(11), 1074-1079, 2010.

X. Jin, and J. Huang. "Adsorption of vanillin by an anisole-modified hyper-cross-linked polystyrene resin from aqueous solution: Equilibrium, kinetics, and dynamics," Advances in Polymer Technology, 32, 1-10, 2012.

G. Q. Xiao, L. P. Long, and J. L. Wang. "Synthesis of the water-compatible p-acetaminophen resin and its adsorption performances for vanillin in aqueous solution," Chinese Chemical Letters, 23(1), 123-126, 2012.

M. I. F. Mota, P. C. R. Pinto, J. M. Loureiro, and A. E. Rodrigues. "Adsorption of vanillin and syringaldehyde onto a macroporous polymeric resin," Chemical Engineering Journal, 288, 869-879, 2016.

R. Ghosh. "Principles Of Bioseparations Engineering," World Scientific, Singapore, 2006.

C. J. Geankoplis. "Transport Processes and Separation Process Principles (Includes Unit Operations)," Fourth ed., Prentice Hall, New Jersey, 2003.

U. Krings, and R. Berger. "Porous polymers for fixed bed adsorption of aroma compounds in fermentation processes," Biotechnology Techniques, 9(1), 19-24, 1995.

D. Couteau, and P. Mathaly. "Fixed-bed purification of ferulic acid from sugar-beet pulp using activated carbon: Optimization studies," Bioresource Technology, 64(1), 17-25, 1998.

T. S. Singh, and K. K. Pant. "Experimental and modelling studies on fixed bed adsorption of As(III) ions from aqueous solution," Separation and Purification Technology, 48(3), 288-296, 2006.

A. Adak, M. Bandyopadhyay, and A. Pal. "Fixed bed column study for the removal of crystal violet (C. I. Basic Violet 3) dye from aquatic environment by surfactant-modified alumina," Dyes and Pigments, 69(3), 245-251, 2006.

R. A. Samah, N. Zainol, P. L. Yee, C. M. Pawing, and S. Abd-Aziz. "Adsorption of Vanillin using Macroporous Resin H103," Adsorption Science & Technology, 31(7), 599-610, 2013.

E.-G. Lee, S.-H. Yoon, A. Das, S.-H. Lee, C. Li, J.-Y. Kim, M.-S. Choi, D.-K. Oh, and S.-W. Kim. "Directing vanillin production from ferulic acid by increased acetyl-CoA consumption in recombinant Escherichia coli," Biotechnology and Bioengineering, 102(1), 200-208, 2009.

M. Goyal, R. Dhawan, and M. Bhagat. "Adsorption of gallic acid from aqueous solution using fixed bed activated carbon columns," Separation Science and Technology, 45(9), 1265-1274, 2010.

Q.-F. Zhang, Z.-T. Jiang, H.-J. Gao, and R. Li. "Recovery of vanillin from aqueous solutions using macroporous adsorption resins," European Food Research and Technology, 226(3), 377-383, 2008.

A. G. Huesgen, Analysis of natural and artificial vanilla preparations, Agilent Application Note, pp. 1-12, 2011.

W. W. Eckenfelder. "Industrial Water Pollution Control," McGraw-Hill, New York, 2000.

P. A. Belter, E. L. Cussler, and W. S. Hu. "Bioseparations: Downstream Processing for Biotechnology," Wiley, New York, 1988.

J. D. Seader, E. J. Henley, and D. K. Roper. "Separation Process Principles," John Wiley & Sons, New Jersey, 2010.

N. Chen, Z. Zhang, C. Feng, M. Li, R. Chen, and N. Sugiura. "Investigations on the batch and fixed-bed column performance of fluoride adsorption by Kanuma mud," Desalination, 268(1–3), 76-82, 2011.

M. Dutta, J. K. Basu, H. FaraZ, N. Gautam, and A. Kumar. "Fixed bed column study of textile dye, direct blue 86 by using a composite adsorbent," Archives of Applied Science Research, 4(2), 882-891, 2012.

G. S. Bohart, and E. Q. Adams. "Some aspects of the behavior of charcoal with respect to chlorine," Journal of the American Chemical Society, 42(3), 523-544, 1920.

B. Kiran, and A. Kaushik. "Cyanobacterial biosorption of Cr(VI): Application of two parameter and Bohart Adams models for batch and column studies," Chemical Engineering Journal, 144(3), 391-399, 2008.

D. C. K. Ko, J. F. Porter, and G. McKay. "Optimised correlations for the fixed-bed adsorption of metal ions on bone char," Chemical Engineering Science, 55(23), 5819-5829, 2000.

K. H. Chu, E. Y. Kim, and X. Feng. "Batch kinetics of metal biosorption: Application of the Bohart-Adams rate law," Separation Science and Technology, 46(10), 1591-1601, 2011.

K. H. Chu. "Improved fixed bed models for metal biosorption," Chemical Engineering Journal, 97(2–3), 233-239, 2004.

B. Volesky, and I. Prasetyo. "Cadmium removal in a biosorption column," Biotechnology and Bioengineering, 43(11), 1010-1015, 1994.

J. M. Brady, J. M. Tobin, and J.-C. Roux. "Continuous fixed bed biosorption of Cu2+ ions: application of a simple two parameter mathematical model," Journal of Chemical Technology & Biotechnology, 74(1), 71-77, 1999.




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